Mayer f-function formalism

E841012

The Mayer f-function formalism is a mathematical framework in statistical mechanics that expresses intermolecular interactions via cluster expansions to analyze the thermodynamic properties of fluids and gases.

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Predicate Object
instanceOf cluster expansion method
statistical mechanics formalism
appliesTo classical fluids
gases
assumes classical distinguishable particles in many applications
pairwise additive interactions in simplest form
basedOn intermolecular pair potential
coreIdea express partition function as sum over clusters
represent interactions via products of f-functions
defines f(r) = exp[-β u(r)] - 1
developedBy Joseph E. Mayer NERFINISHED
Maria Goeppert-Mayer NERFINISHED
field statistical mechanics
generalizedTo quantum cluster expansions
influenced diagrammatic methods in many-body physics
integral equation theories of liquids
modern liquid state theory
introducesConcept Mayer f-function
leadsTo cluster integrals
virial coefficients
limitation convergence issues at high density
mathematicalTool graph theory
relatedConcept Mayer cluster expansion NERFINISHED
diagrammatic cluster representation
relatedTo canonical ensemble
grand canonical ensemble
relatesQuantity interparticle distance r
inverse temperature β
pair potential u(r)
representsBondsAs Mayer f-functions
representsClustersAs graphs
representsParticlesAs graph vertices
timePeriod 1930s
usedFor analysis of non-ideal gas behavior
calculation of chemical potential
calculation of free energy
calculation of pressure from microscopic interactions
calculation of thermodynamic properties
cluster expansion of the partition function
low-density expansions of fluids
virial expansion of the equation of state
usedIn derivation of virial equation of state
usesSymbol f(r)
u(r)
β
validRegime low to moderate densities

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Joseph Edward Mayer notableWork Mayer f-function formalism