Huang–Rhys factor

E27438

The Huang–Rhys factor is a dimensionless parameter in solid-state and molecular spectroscopy that quantifies the strength of electron–phonon (vibronic) coupling during electronic transitions.

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Statements (48)

Predicate Object
instanceOf dimensionless physical quantity
spectroscopic parameter
appearsIn Poisson distribution of phonon sideband intensities
appliesTo color centers in crystals
defect centers in solids
electronic transitions
molecular electronic spectra
optical absorption
photoluminescence
dependsOn displacement between ground and excited state potential energy surfaces
effective phonon mode energy
determines relative intensity of phonon sidebands
relative intensity of vibronic peaks
weight of zero-phonon line
estimatedFrom fit to vibronic sideband intensities
temperature dependence of luminescence
field molecular spectroscopy
optical spectroscopy
solid-state physics
governs relative probability of n-phonon transitions
hasProperty dimensionless
influences Debye–Waller factor
Stokes shift
shape of optical absorption spectra
shape of optical emission spectra
introducedBy A. M. Rhys
Kun Huang
mathematicalRole average number of phonons involved in an electronic transition
quantifies electron–phonon coupling strength
vibronic coupling strength
relatedTo Franck–Condon principle
surface form: Franck–Condon factors

Franck–Condon principle
phonon sidebands
vibronic progression
zero-phonon line
symbol S
typicalRange much less than 1 for weak coupling
of order 1 or larger for strong coupling
usedIn color center spectroscopy
nitrogen-vacancy center spectroscopy
organic molecular crystals
quantum emitter characterization
rare-earth ion spectroscopy
semiconductor defect spectroscopy
single-molecule spectroscopy
usedInModel configuration coordinate model
harmonic oscillator approximation
yearProposed 1950

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Franck–Condon principle relatedTo Huang–Rhys factor